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USGS2021

Anomalous noble gas solubility in liquid cloud water: Possible implications for noble gas temperatures and cloud physics

The noble gas temperature climate proxy is an established tool that has previously been applied to determine the source of groundwater recharge, however, unanswered questions remain. In fractured media (e.g., volcanic islands) recharge can be so rapid that groundwater is significantly depleted in heavy noble gases, indicating that the water has retained noble gas concentrations from higher elevations. Previous studies of rain samples have confirmed a match to patterns seen in fractured-rock groundwater for heavy noble gases along with a significant helium excess. Snow has been shown to be a credible source for both the helium excess and the observed heavy noble gas pattern. Here, liquid cloud water samples were collected at two mountainous sites and analyzed for noble gas concentrations. A pattern like that of rainwater was found. However, an analysis of diffusive uptake of noble gases into cloud water demonstrates that droplets of 1 mm diameter and smaller should be in constant solubility equilibrium with the atmosphere. To explain this, we present a novel hypothesis that relies on the assumption that liquid water consists of two types of water molecule clusters bounded by hydrogen bonds: a low-density ice-like structure and a high-density condensed structure. In this model, the pressure gradient near the surface of a droplet resulting from surface tension could allow for the formation of a surface layer that is rich in ice-like low density clusters. This can explain both the helium excess and the heavy noble gas depletion seen in the samples.

Puerto Rico↗

USGS2019

Application of an updated atmospheric model to explore volcano infrasound propagation and detection in Alaska

Winds and temperature gradients greatly affect the long-range propagation of infrasound . The spatio-temporal variability of these parameters must therefore be accurately characterized to correctly interpret recorded infrasound at long distances, specifically to differentiate between source and propagation effects. Here we present the first results of an open source reanalysis model, termed Alaska Volcano Observatory Ground-to-Space (AVO-G2S), constructed to accurately characterize the atmosphere and model long-range infrasound propagation from volcanic eruptions in Alaska. We select a number of case studies to examine recent eruptions of Alaskan volcanoes whose ash emissions posed a threat to air traffic, including the two most recent eruptions of Pavlof Volcano and two typical explosions from Cleveland Volcano. Strong tropospheric ducting and low noise at the station during the 21 July 2015 explosion of Cleveland Volcano led to an automated detection of the explosion at an infrasound array 992 km away, whereas low signal-to-noise ratio for the 6 November 2014 Cleveland Volcano explosion helps explain the non-detection in real-time of a predicted strong stratospheric arrival. For the November 2014 Pavlof eruption, discrepancies between local seismic data and a distal infrasound array 460 km away cannot be solely explained by changes in atmospheric conditions, though some features of the complex propagation predictions follow the trends in long-range infrasound signals. The most recent eruption of Pavlof Volcano in March 2016 shows minimal changes in propagation conditions throughout the eruption and therefore indicates that the signals detected at long-range primarily reflect source processes. These results show how detailed examination of the acoustic propagation conditions provides insight into detection capability and eruption dynamics. Future work will implement AVO-G2S and high-resolution long-range infrasound propagation modeling in real-time for Alaskan volcanoes of interest.

Alaska↗

USGS2011

Measurements of Martian dust devil winds with HiRISE

We report wind measurements within Martian dust devils observed in plan view from the High Resolution Imaging Science Experiment (HiRISE) orbiting Mars. The central color swath of the HiRISE instrument has three separate charge‐coupled devices (CCDs) and color filters that observe the surface in rapid cadence. Active features, such as dust devils, appear in motion when observed by this region of the instrument. Our image animations reveal clear circulatory motion within dust devils that is separate from their translational motion across the Martian surface. Both manual and automated tracking of dust devil clouds reveal tangential winds that approach 20–30 m s −1 in some cases. These winds are sufficient to induce a ∼1% decrease in atmospheric pressure within the dust devil core relative to ambient, facilitating dust lifting by reducing the threshold wind speed for particle elevation. Finally, radial velocity profiles constructed from our automated measurements test the Rankine vortex model for dust devil structure. Our profiles successfully reveal the solid body rotation component in the interior, but fail to conclusively illuminate the profile in the outer regions of the vortex. One profile provides evidence for a velocity decrease as a function of r −1/2 , instead of r −1 , suggestive of surface friction effects. However, other profiles do not support this observation, or do not contain enough measurements to produce meaningful insights.

Geophysical Research Letters↗

USGS2009

Inventories and mobilization of unsaturated zone sulfate, fluoride, and chloride related to land use change in semiarid regions, southwestern United States and Australia

Unsaturated zone salt reservoirs are potentially mobilized by increased groundwater recharge as semiarid lands are cultivated. This study explores the amounts of pore water sulfate and fluoride relative to chloride in unsaturated zone profiles, evaluates their sources, estimates mobilization due to past land use change, and assesses the impacts on groundwater quality. Inventories of water‐extractable chloride, sulfate, and fluoride were determined from borehole samples of soils and sediments collected beneath natural ecosystems ( N = 4), nonirrigated (“rain‐fed”) croplands ( N = 18), and irrigated croplands ( N = 6) in the southwestern United States and in the Murray Basin, Australia. Natural ecosystems contain generally large sulfate inventories (7800–120,000 kg/ha) and lower fluoride inventories (630–3900 kg/ha) relative to chloride inventories (6600–41,000 kg/ha). Order‐of‐magnitude higher chloride concentrations in precipitation and generally longer accumulation times result in much larger chloride inventories in the Murray Basin than in the southwestern United States. Atmospheric deposition during the current dry interglacial climatic regime accounts for most of the measured sulfate in both U.S. and Australian regions. Fluoride inventories are greater than can be accounted for by atmospheric deposition in most cases, suggesting that fluoride may accumulate across glacial/interglacial climatic cycles. Chemical modeling indicates that fluorite controls fluoride mobility and suggests that water‐extractable fluoride may include some fluoride from mineral dissolution. Increased groundwater drainage/recharge following land use change readily mobilized chloride. Sulfate displacement fronts matched or lagged chloride fronts by up to 4 m. In contrast, fluoride mobilization was minimal in all regions. Understanding linkages between salt inventories, increased recharge, and groundwater quality is important for quantifying impacts of anthropogenic activities on groundwater quality and is required for remediating salinity problems.

Water Resources Research↗

USGS2017

Broadband seismic noise attenuation versus depth at the Albuquerque Seismological Laboratory

Seismic noise induced by atmospheric processes such as wind and pressure changes can be a major contributor to the background noise observed in many seismograph stations, especially those installed at or near the surface. Cultural noise such as vehicle traffic or nearby buildings with air handling equipment also contributes to seismic background noise. Such noise sources fundamentally limit our ability to resolve earthquake‐generated signals. Many previous seismic noise versus depth studies focused separately on either high‐frequency ( > 1    Hz "> > 1 Hz ) or low‐frequency ( < 0.05    Hz "> < 0.05 Hz ) bands. In this study, we use modern high‐quality broadband (BB) and very broadband (VBB) seismometers installed at depths ranging from 1.5 to 188 m at the Albuquerque Seismological Laboratory to evaluate noise attenuation as a function of depth over a broad range of frequencies (0.002–50 Hz). Many modern seismometer deployments use BB or VBB seismometers installed at various depths, depending on the application. These depths range from one‐half meter or less in aftershock study deployments, to one or two meters in the Incorporated Research Institutions for Seismology Transportable Array (TA), to a few meters (shallow surface vaults) up to 100 m or more (boreholes) in the permanent observatories of the Global Seismographic Network (GSN). It is important for managers and planners of these and similar arrays and networks of seismograph stations to understand the attenuation of surface‐generated noise versus depth so that they can achieve desired performance goals within their budgets as well as their frequency band of focus. The results of this study will assist in decisions regarding BB and VBB seismometer installation depths. In general, we find that greater installation depths are better and seismometer emplacement in hard rock is better than in soil. Attenuation for any given depth varies with frequency. More specifically, we find that the dependence of depth will be application dependent based on the frequency band and sensitive axes of interest. For quick deployments (like aftershock studies), 1 m may be deep enough to produce good data, especially when the focus is on vertical data where temperature stability fundamentally limits the low‐frequency noise levels and little low‐frequency data will be used. For temporary (medium‐term) deployments (e.g., TA) where low cost can be very important, 2–3 m should be sufficient, but such shallow installations will limit the ability to resolve low‐frequency signals, especially on horizontal components. Of course, one should try for maximum burial depth within the budget when there is interest in using the data for low‐frequency applications. For long‐term deployments like the permanent observatories of the GSN and similar networks, 100–200 m depth in hard rock is desirable to achieve lowest noise, although 30–60 m may be acceptable.

Bulletin of the Seismological Society of America↗

USGS2020

Ecological forecasting—21st century science for 21st century management

Natural resource managers are coping with rapid changes in both environmental conditions and ecosystems. Enabled by recent advances in data collection and assimilation, short-term ecological forecasting may be a powerful tool to help resource managers anticipate impending near-term changes in ecosystem conditions or dynamics. Managers may use the information in forecasts to minimize the adverse effects of ecological stressors and optimize the effectiveness of management actions. To explore the potential for ecological forecasting to enhance natural resource management, the U.S. Geological Survey (USGS) convened a workshop titled "Building Capacity for Applied Short-Term Ecological Forecasting" on May 29—31, 2019, with participants from several Federal agencies, including the Bureau of Land Management, the U.S. Fish and Wildlife Service, the National Park Service, and the National Oceanic and Atmospheric Administration as well as all mission areas within the USGS. Participants broadly agreed that short-term ecological forecasting—on the order of days to years into the future—has tremendous potential to improve the quality and timeliness of information available to guide resource management decisions. Participants considered how ecological forecasting could directly affect their agency missions and specified numerous critical tools for addressing natural resource management concerns in the 21st century that could be enhanced by ecological forecasting. Given this breadth of possible applications for forecast products, participants developed a repeatable framework for evaluating potential value of a forecast product for enhancing resource management. Applying that process to a large list of forecast ideas that were developed in a brainstorming session, participants identified a small set of promising forecast products that illustrate the value of ecological forecasting for informing resource management. Workshop outcomes also include insights about important likely obstacles and next steps. In particular, reliable production and delivery of operational ecological forecasts will require a sustained commitment by research agencies, in partnership with resource management agencies, to maintain and improve forecasting tools and capabilities.

Open-File Report↗

USGS2024

Dust in the Critical Zone: North American case studies

The dust cycle facilitates the exchange of particles among Earth's major systems, enabling dust to traverse ecosystems, cross geographic boundaries, and even move uphill against the natural flow of gravity. Dust in the atmosphere is composed of a complex and ever-changing mixture that reflects the evolving human footprint on the landscape. The emission, transport, and deposition of dust interacts with and connects Critical Zone processes at all spatial and temporal scales. Landscape properties, land use, and climatic factors influence the wind erosion of soil and nutrient loss, which alters the long-term ecological dynamics at erosional locations. Once in the atmosphere, dust particles influence the amount of solar radiation reaching Earth, and interact with longwave (terrestrial) radiation, with cascading effects on the climate system. Finally, the wet and dry deposition of particles influences ecosystem structure, composition, and function over both short and long-term scales. Tracking dust particles from source to sink relies on monitoring and measurement of the geochemical composition and size distribution of the particles, space-borne and ground-based remote sensing, and dust modeling. Dust is linked to human systems via land use and policies that contribute to dust emissions and the health-related consequences of particulate loads and composition. Despite the significant influence dust has in shaping coupled natural-human systems, it has not been considered a key component of the Critical Zone. Here, we demonstrate that dust particles should be included as a key component of the Critical Zone by outlining how dust interacts with and shapes Earth System processes from generation, through transport, to deposition. We synthesize current understanding from global research and identify critical data and knowledge gaps while showcasing case studies from North America.

Earth-Science Reviews↗

USGS2010

Controls on mangrove forest‐atmosphere carbon dioxide exchanges in western Everglades National Park

We report on net ecosystem production (NEP) and key environmental controls on net ecosystem exchange (NEE) of carbon dioxide (CO 2 ) between a mangrove forest and the atmosphere in the coastal Florida Everglades. An eddy covariance system deployed above the canopy was used to determine NEE during January 2004 through August 2005. Maximum daytime NEE ranged from −20 to −25 μ mol (CO 2 ) m −2 s −1 between March and May. Respiration (R d ) was highly variable (2.81 ± 2.41 μ mol (CO 2 ) m −2 s −1 ), reaching peak values during the summer wet season. During the winter dry season, forest CO 2 assimilation increased with the proportion of diffuse solar irradiance in response to greater radiative transfer in the forest canopy. Surface water salinity and tidal activity were also important controls on NEE. Daily light use efficiency was reduced at high (>34 parts per thousand (ppt)) compared to low (<17 ppt) salinity by 46%. Tidal inundation lowered daytime R d by ∼0.9 μ mol (CO 2 ) m −2 s −1 and nighttime R d by ∼0.5 μ mol (CO 2 ) m −2 s −1 . The forest was a sink for atmospheric CO 2 , with an annual NEP of 1170 ± 127 g C m −2 during 2004. This unusually high NEP was attributed to year‐round productivity and low ecosystem respiration which reached a maximum of only 3 g C m −2 d −1 . Tidal export of dissolved inorganic carbon derived from belowground respiration likely lowered the estimates of mangrove forest respiration. These results suggest that carbon balance in mangrove coastal systems will change in response to variable salinity and inundation patterns, possibly resulting from secular sea level rise and climate change.

Florida↗

USGS2024

Hydroacoustic observations reveal drivers of mixing and salinization of a karst subterranean estuary during intense precipitation

Karst subterranean estuaries within globally ubiquitous carbonate aquifers are coastal groundwater ecosystems that provide an essential water resource for human populations. To understand the drivers of salinization within a coastal aquifer in the Yucatan Peninsula (Mexico), we employed hydroacoustics in flooded caves to observe how oceanic and atmospheric events facilitate mixing between the meteoric lens (fresh-brackish groundwater) and the saline groundwater on tidal and episodic timescales. Precipitation during Tropical Storm Carlotta increased the flow and salinity of the meteoric lens without evidence for vertical mixing across the halocline. We postulate that vertical migration of haloclines in the conduit relative to those within the rock matrix during precipitation creates lateral density gradients that drive mixing, and ultimately creates a brackish layer within the meteoric lens. These results provide a mechanistic explanation for vertical and lateral exchange in a coastal carbonate aquifer, which has implications for groundwater response to future climatic change.

Ox Bel Ha cave system, Yucatan peninsula↗

USGS2018

Variation in soil carbon dioxide efflux at two spatial scales in a topographically complex boreal forest

Carbon dynamics of high-latitude regions are an important and highly uncertain component of global carbon budgets, and efforts to constrain estimates of soil-atmosphere carbon exchange in these regions are contingent on accurate representations of spatial and temporal variability in carbon fluxes. This study explores spatial and temporal variability in soilatmosphere carbon dynamics at both fine and coarse spatial scales in a high-elevation, permafrost-dominated boreal black spruce forest. We evaluate the importance of landscape-level investigations of soil-atmosphere carbon dynamics by characterizing seasonal trends in soil-atmosphere carbon exchange, describing soil temperature-moisture-respiration relations, and quantifying temporal and spatial variability at two spatial scales: the plot scale (0–5 m) and the landscape scale (500–1000 m). Plot-scale spatial variability (average variation on a given measurement day) in soil CO 2 efflux ranged from a coefficient of variation (CV) of 0.25 to 0.69, and plot-scale temporal variability (average variation of plots across measurement days) in efflux ranged from a CV of 0.19 to 0.36. Landscape-scale spatial and temporal variability in efflux was represented by a CV of 0.40 and 0.31, respectively, indicating that plot-scale spatial variability in soil respiration is as great as landscape-scale spatial variability at this site. While soil respiration was related to soil temperature at both the plot- and landscape scale, landscape-level descriptions of soil moisture were necessary to define soil respiration-moisture relations. Soil moisture variability was also integral to explaining temporal variability in soil respiration. Our results have important implications for research efforts in high-latitude regions where remote study sites make landscape-scale field campaigns challenging.

Arctic, Antarctic, and Alpine Research↗

USGS1998

Tracing solute mobility at the Panola Mountain Research Watershed, Georgia, USA: Variations in Na+, Cl-, and H4SiO4 concentrations

Concentration variations of sodium (N+). chloride (Cl-). and dissolved silica (H4SiO4) in rainfall, throughfall, soil water, groundwater and streamwater were evaluated at the Panola Mountain Research Watershed near Atlanta, Georgia, to determine how variations in concentrations of these solutes provide greater understanding of water quality evolution at the hillslope and catchment scales Stormwater moves rapidly to depth along preferred pathways in a deciduous forest hillslope, but the composition of the mobile unsaturated zone water in the hillslope is not reflected in compositional variations of streamwater during rainstorms. The Na+, Cl-, and H4SiO4 concentrations behave similarly in streamwater, decreasing with increasing discharge and increasing with water residence time. Consequently, the lowest flows are associated with the highest concentrations and the oldest water. Streamwater composition is most similar to groundwater and stormflow variations reflect a dilution of groundwater. Subtle differences in the relations among solute concentrations and discharge reflect different sources, especially for Cl-. For example, the residence time of groundwater, as inferred from landscape position, generally is positively related to Na+ and H4SiO4 concentrations, but not to Cl- concentrations. The Na+ and H4SiO4 are derived from mineral weathering and are continuously supplied along hydrological pathways. In contrast, Cl- is derived from atmospheric deposition and is affected only by evapotranspiration (ET) and transport. ET increases Cl- concentrations in matrix soil waters, which are subsequently transported to the saturated zone where Cl- is effectively isolated from further evaporative concentration.

IAHS-AISH Publication↗

USGS2013

Ocean climate indicators: A monitoring inventory and plan for tracking climate change in the north-central California coast and ocean region

The impacts of climate change, defined as increasing atmospheric and oceanic carbon dioxide and associated increases in average global temperature and oceanic acidity, have been observed both globally and on regional scales, such as in the North-central California coast and ocean, a region that extends from Point Arena to Point Año Nuevo and includes the Pacific coastline of the San Francisco Bay Area. Because of the high economic and ecological value of the region’s marine environment, the Gulf of the Farallones National Marine Sanctuary (GFNMS) and other agencies and organizations have recognized the need to evaluate and plan for climate change impacts. Climate change indicators can be developed on global, regional, and site-specific spatial scales, and they provide information about the presence and potential impacts of climate change. While indicators exist for the nation and for the state of California as a whole, no system of ocean climate indicators exist that specifically consider the unique characteristics of the California coast and ocean region. To that end, GFNMS collaborated with over 50 regional, federal, and state natural resource managers, research scientists, and other partners to develop a set of 2 ocean climate indicators specific to this region. A smaller working group of 13 regional partners developed monitoring goals, objectives, strategies, and activities for the indicators and recommended selected species for biological indicators, resulting in the Ocean Climate Indicators Monitoring Inventory and Plan. The working group considered current knowledge of ongoing monitoring, feasibility of monitoring, costs, and logistics in selecting monitoring activities and selected species.

Report↗

USGS2015

Water-quality assessment of the Lower Grand River Basin, Missouri and Iowa, USA, in support of integrated conservation practices

The effectiveness of agricultural conservation programmes to adequately reduce nutrient exports to receiving streams and to help limit downstream hypoxia issues remains a concern. Quantifying programme success can be difficult given that short-term basin changes may be masked by long-term water-quality shifts. We evaluated nutrient export at stream sites in the 44 months that followed a period of increased, integrated conservation implementation within the Lower Grand River Basin. These short-term responses were then compared with export that occurred in the main stem and adjacent rivers in northern Missouri over a 22-year period to better contextualize any recent changes. Results indicate that short-term (October 2010 through May 2014) total nitrogen (TN) concentrations in the Grand River were 20% less than the long-term average, and total phosphorus (TP) concentrations were 23% less. Nutrient reductions in the short term were primarily the result of the less-than-average precipitation and, consequently, streamflow that was 36% below normal. Therefore, nutrient concentrations measured in tributary streams were likely less than normal during the implementation period. Northern Missouri streamflow-normalized TN concentrations remained relatively flat or declined over the period 1991 through 2013 likely because available sources of nitrogen, determined as the sum of commercial fertilizers, available animal manures and atmospheric inputs, were typically less than crop requirement for much of that time frame. Conversely, flow-normalized stream TP concentrations increased over the past 22 years in northern Missouri streams, likely in response to many years of phosphorus inputs in excess of crop requirements. Stream nutrient changes were most pronounced during periods that coincided with the major tillage, planting and growth phases of row crops and increased streamflow. Nutrient reduction strategies targeted at the period February through June would likely have the greatest impact on reducing nutrient export from the basin. Published 2015. This article is a U.S. Government work and is in the public domain in the USA.

River Research and Applications↗

USGS2007

Warming may create substantial water supply shortages in the Colorado River basin

The high demand for water, the recent multiyear drought (1999-2007), and projections of global warming have raised questions about the long-term sustainability of water supply in the southwestern United States. In this study, the potential effects of specific levels of atmospheric warming on water-year streamflow in the Colorado River basin are evaluated using a water-balance model, and the results are analyzed within the context of a multi-century tree-ring reconstruction (1490-1998) of streamflow for the basin. The results indicate that if future warming occurs in the basin and is not accompanied by increased precipitation, then the basin is likely to experience periods of water supply shortages more severe than those inferred from the longterm historical tree-ring reconstruction. Furthermore, the modeling results suggest that future warming would increase the likelihood of failure to meet the water allocation requirements of the Colorado River Compact.

Geophysical Research Letters↗

USGS1973

Catalog of earthquakes along the San Andreas fault system in Central California, April-June 1972

Numerous small earthquakes occur each day in the coast ranges of Central California. The detailed study of these earthquakes provides a tool for gaining insight into the tectonic and physical processes responsible for the generation of damaging earthquakes. This catalog contains the fundamental parameters for earthquakes located within and adjacent to the seismograph network operated by the National Center for Earthquake Research (NCER), U.S. Geological Survey, during the period April - June, 1972. The motivation for these detailed studies has been described by Pakiser and others (1969) and by Eaton and others (1970). Similar catalogs of earthquakes for the years 1969, 1970 and 1971 have been prepared by Lee and others (1972 b, c, d). A catalog for the first quarter of 1972 has been prepared by Wesson and others (1972). The basic data contained in these catalogs provide a foundation for further studies. This catalog contains data on 910 earthquakes in Central California. A substantial portion of the earthquakes reported in this catalog represents a continuation of the sequence of earthquakes in the Bear Valley area which began in February, 1972 (Wesson and others, 1972). Arrival times at 126 seismograph stations were used to locate the earthquakes listed in this catalog. Of these, 101 are telemetered stations operated by NCER. Readings from the remaining 25 stations were obtained through the courtesy of the Seismographic Stations, University of California, Berkeley (UCB); the Earthquake Mechanism Laboratory, National Oceanic and Atmospheric Administration, San Francisco (EML); and the California Department of Water Resources, Sacramento. The Seismographic Stations of the University of California, Berkeley, have for many years published a bulletin describing earthquakes in Northern California and the surrounding area, and readings at UCB Stations from more distant events. The purpose of the present catalog is not to replace the UCB Bulletin, but rather to supplement it, by describing the seismicity of a portion of central California in much greater detail.

California↗

USGS2017

Terrestrial ecosystem model performance in simulating productivity and its vulnerability to climate change in the northern permafrost region

Realistic projection of future climate-carbon (C) cycle feedbacks requires better understanding and an improved representation of the C cycle in permafrost regions in the current generation of Earth system models. Here we evaluated 10 terrestrial ecosystem models for their estimates of net primary productivity (NPP) and responses to historical climate change in permafrost regions in the Northern Hemisphere. In comparison with the satellite estimate from the Moderate Resolution Imaging Spectroradiometer (MODIS; 246 ± 6 g C m −2 yr −1 ), most models produced higher NPP (309 ± 12 g C m −2 yr −1 ) over the permafrost region during 2000–2009. By comparing the simulated gross primary productivity (GPP) with a flux tower-based database, we found that although mean GPP among the models was only overestimated by 10% over 1982–2009, there was a twofold discrepancy among models (380 to 800 g C m −2 yr −1 ), which mainly resulted from differences in simulated maximum monthly GPP (GPP max ). Most models overestimated C use efficiency (CUE) as compared to observations at both regional and site levels. Further analysis shows that model variability of GPP and CUE are nonlinearly correlated to variability in specific leaf area and the maximum rate of carboxylation by the enzyme Rubisco at 25°C ( V c max_25 ), respectively. The models also varied in their sensitivities of NPP, GPP, and CUE to historical changes in climate and atmospheric CO 2 concentration. These results indicate that model predictive ability of the C cycle in permafrost regions can be improved by better representation of the processes controlling CUE and GPP max as well as their sensitivity to climate change.

Journal of Geophysical Research: Biogeosciences↗

USGS2016

Variation of organic matter quantity and quality in streams at Critical Zone Observatory watersheds

The quantity and chemical composition of dissolved organic matter (DOM) in surface waters influence ecosystem processes and anthropogenic use of freshwater. However, despite the importance of understanding spatial and temporal patterns in DOM, measures of DOM quality are not routinely included as part of large-scale ecosystem monitoring programs and variations in analytical procedures can introduce artifacts. In this study, we used consistent sampling and analytical methods to meet the objective of defining variability in DOM quantity and quality and other measures of water quality in streamflow issuing from small forested watersheds located within five Critical Zone Observatory sites representing contrasting environmental conditions. Results show distinct separations among sites as a function of water quality constituents. Relationships among rates of atmospheric deposition, water quality conditions, and stream DOM quantity and quality are consistent with the notion that areas with relatively high rates of atmospheric nitrogen and sulfur deposition and high concentrations of divalent cations result in selective transport of DOM derived from microbial sources, including in-stream microbial phototrophs. We suggest that the critical zone as a whole strongly influences the origin, composition, and fate of DOM in streams. This study highlights the value of consistent DOM characterization methods included as part of long-term monitoring programs for improving our understanding of interactions among ecosystem processes as controls on DOM biogeochemistry.

Water Resources Research↗

USGS2008

Physical property changes in hydrate-bearing sediment due to depressurization and subsequent repressurization

Physical property measurements of sediment cores containing natural gas hydrate are typically performed on material exposed, at least briefly, to non-in situ conditions during recovery. To examine the effects of a brief excursion from the gas-hydrate stability field, as can occur when pressure cores are transferred to pressurized storage vessels, we measured physical properties on laboratory-formed sand packs containing methane hydrate and methane pore gas. After depressurizing samples to atmospheric pressure, we repressurized them into the methane-hydrate stability field and remeasured their physical properties. Thermal conductivity, shear strength, acoustic compressional and shear wave amplitudes, and speeds of the original and depressurized/repressurized samples are compared. X– ray computed tomography images track how the gas-hydrate distribution changes in the hydrate-cemented sands owing to the depressurizaton/repressurization process. Because depressurization-induced property changes can be substantial and are not easily predicted, particularly in water-saturated, hydrate-bearing sediment, maintaining pressure and temperature conditions throughout the core recovery and measurement process is critical for using laboratory measurements to estimate in situ properties.

Journal of Geophysical Research B: Solid Earth↗