USGS · 70027725
CO 2 mitigation via accelerated limestone weathering
Abstract
We evaluate accelerated weathering of limestone (AWL: CO 2 + CaCO 3 + H 2 O=> Ca 2+ + 2HCO 3 - ) as a low-tech, inexpensive, high-capacity, environmentally-friendly CO 2 capture and sequestration technology. With access to seawater and limestone being essential to this approach, significant limestone resources are close to most CO 2 -emitting power plants along the coastal US. Waste fines, representing more than 20% of current US crushed limestone production (>10 9 tonnes/yr), could be used as an inexpensive source of AWL carbonate. Under such circumstances CO 2 mitigation cost could be as low as $3-$4/tonne. More broadly, 10-20% of US point-source CO 2 emissions could be treated at $20-$30/tonne CO 2 . AWL end-solution disposal in the ocean would significantly reduce effects on ocean pH and carbonate chemistry relative to those caused by direct atmospheric or ocean CO 2 disposal. Indeed, the increase in ocean Ca 2+ and bicarbonate offered by AWL should enhance growth of corals and other calcifying marine organisms.
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Greg H. Rau, Kevin G. Knauss, William H. Langer, Caldeira. 2004. CO 2 mitigation via accelerated limestone weathering. https://pubs.usgs.gov/publication/70027725
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